Psychopaths, occasionally also called Sociopaths, are villains associated with antisocial personality disorder, otherwise known as psychopathy. They show traits and symptoms of antisocial personality disorder, narcissistic personality disorder, or paranoid personality disorder.
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- Sabine Moreau
- Sadistic Claus
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- Salacious B. Crumb
- Scar
- Scott Lavin
- Sean Ambrose
- Sean Keanan
- Selim Bradley
- Shan Yu
- Shaw
- Sheldon J. Plankton
- Shin Hati
- Shishio Makoto
- Shou Tucker
- Shredder (2012 TMNT)
- Shuu Tsukiyama
- Sideshow Bob
- Slade
- Smaug
- Snack-Stealing Squirrel
- Solomon Lane
- Spinel
- Squeezy Squirrel
- Starfire (Teen Titans Go!)
- Stinky Pete
- Sue (The Loud House)
- Sunset Shimmer
- Surtr (Legend of the Guardians)
- Sweeney Todd (The Demon Barber of Fleet Street)
- Syndrome
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- Takako Sugiura
- Tammy Jane
- Tate Langdon
- Thanos (Marvel: Ultimate Alliance)
- The Addams Family
- The Chameleon
- The Hitchhiker
- The Joker
- The Storm King
- Thing
- Thing (Wednesday)
- Thomas LeBlanc
- Thrax (Osmosis Jones)
- Thunderclap
- Tiger Claw
- Tiger General
- Tolga Trunkov
- Tomohiko Kazami
- Tony Trihull
- Tubbs Pacer
- Tyler Gremlin
- Tyrone King
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